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zeolite naa, the diffusion rates decrease in a monotonic fashion as the carbon chain length increases, as might be expected. however, this does contrast the behaviour of n-alkanes adsorbed.
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computational high-throughput screening was carried out to assess a large number of experimentally reported metalorganic frameworks and zeolites for their utility in hexane isomer separation. through the work, we identified many mofs and zeolites with high selectivity for the group of n-hexane, 2-methylpentane, and 3-methylpentane versus .
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the confinement effects due to the constraints of the zeolite micropores can manifest in destabilization of the TS and the product site-h CH states. the former scenario is realized when the zeolite walls exert geometrical constraints to CH approaching the reactive o-center, resulting in the effective destabilization of the .
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molecular simulations with periodic boundary conditions require the definition of a certain cutoff radius, rc, beyond which pairwise dispersion interactions are neglected. for the simulation of homogeneous phases the use of tail corrections is well-established, which can remedy this truncation of the potential. these corrections are built under the assumption that beyond rc the radial .
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from this fields start to the present, the simple extended coordination compound prussian blue was known since the early century, a porous coordination polymer cuc was reported in 1990, and yaghi and co-workers reported a robust mof with permanent porosity, mof-5, constructed from Zn clusters and linear dicarboxylate linkers in 1999.
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